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Lithium diffusion pathway in Li 1-x Ni 1+x O 2 with the α-NaFeO 2 structure was elucidated using neutron diffraction measurements at high temperatures. In the layered structure of space group R3m, lithium and nickel ions occupy the octahedral 3a and 3b sites, respectively, at room temperature. Above 493 K, a part of lithium shifted from the 3a site...
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