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The gas-phase epoxidation of propylene was studied over MoOx/SiO2 catalysts in a reaction system with a post-catalytic bed volume. In the reaction of a mixture of propylene and propane with oxygen below 578 K, propylene oxide (PO) was mainly formed from the oxidation of propylene. It was found that the oxidation reaction was very sensitive to the temperature of the post-catalytic space more than...
A new catalytic system consisting of titanium oxide clusters supported on silica was found for radical production at relatively low temperature (~573 K). The clusters give rise to selective oxidation products, such as propylene oxide, through gas-phase chain reactions.
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