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Oxidation Catalysts
In article number 2211260, Javier Pérez‐Ramírez and co‐workers report the design of a novel atomically dispersed Mn catalyst on CeO2 for selective oxidation of ammonia to nitrous oxide. Effective stabilization of low‐valence isolated manganese sites results in the formation of a unique catalytic ensemble, which enables facile oxygen activation and leads to unprecedented activity...
Nitrous oxide, N2O, exhibits unique reactivity in oxidation catalysis, but the high manufacturing costs limit its prospective uses. Direct oxidation of ammonia, NH3, to N2O can ameliorate this issue but its implementation is thwarted by suboptimal catalyst selectivity and stability, and the lack of established structure–performance relationships. Systematic and controlled material nanostructuring...
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