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Single‐atom catalysts have become a hot spot because of the high atom utilization efficiency and excellent activity. However, the effect of the support structure in the single‐atom catalyst is often unnoticed in the catalytic process. Herein, a series of carbon spheres supported Ni–N4 single‐atom catalysts with different support structures are successfully synthesized by the fine adjustment of synthetic...
In article number 2003943, Hongfang Li, Rong Cao, and co‐workers successfully synthesize a hollow mesoporous carbon sphere loaded Ni–N4 single‐atom catalyst that exhibits superior catalytic activity toward CO2 electrocatalytic reduction. The geometrical structure of carbon support is verified to affect the CO2 reduction reaction performance greatly. The ultrathin carbon shell and the 7–10 nm mesopores...
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