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Tandem catalysis is a promising way to break the limitation of linear scaling relationship for enhancing efficiency, and the desired tandem catalysts for electrochemical CO2 reduction reaction (CO2RR) are urgent to be developed. Here, a tandem electrocatalyst created by combining Cu foil (CF) with a single‐site Cu(II) metal–organic framework (MOF), named as Cu–MOF–CF, to realize improved electrochemical...
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