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Layered bulk crystals are amenable to exfoliation to yield 2D nanosheets through isolation and intercalation processes, which could be further converted to 1D nanoscale structures. The latter inherit gross morphological and physical properties associated with the precursor structures. Herein, we report three purine‐based crystal structures 1, 2, and 3, where 3 is obtained by a single‐crystal‐to‐single‐crystal...
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