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Metallfreie Photokatalysatoren für die H2‐Entwicklung mit sichtbarem Licht sind wünschenswert für die preisgünstige Energiegewinnung. K. Takanabe und Mitarbeiter stellen in ihrer Zuschrift auf S. 11181 ff. eine Familie kristalliner Kohlenstoffnitride (CNs) durch supramolekulare Aggregation und Polykondensation in einer Salzschmelze her. Diese Photokatalysatoren können über die Menge und Anordnung...
Described herein is the photocatalytic hydrogen evolution using crystalline carbon nitrides (CNs) obtained by supramolecular aggregation followed by ionic melt polycondensation (IMP) using melamine and 2,4,6‐triaminopyrimidine as a dopant. The solid state NMR spectrum of 15N‐enriched CN confirms the triazine as a building unit. Controlling the amount and arrangements of dopants in the CN structure...
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