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A novel semiconductive Co/Fe‐MOF embedded with Fe2O3 nanocrystals (Fe2O3@CoFe‐MOF) is developed as a trifunctional electrocatalyst for the urea oxidation reaction (UOR), oxygen evolution reaction (OER), and hydrogen evolution reaction for enhancing the efficiency of the hydrogen production via the urea‐assisted overall water splitting. Fe2O3@CoFe‐TPyP‐MOF comprises unsaturated metal‐nitrogen coordination...
Nanocrystals play a key role in the modern energy, catalysis, semiconductor, and biology industries due to their unique structures and performances. However, controllable fabrication of ideal nanocrystals with the desired structures and properties is still challenging, which needs a deep understanding of their nucleation and growth process. Here, the research on nucleation and growth of nanocrystals...
An n‐n type heterojunction comprising with CuN and BN dual active sites is synthesized via in situ growth of a conductive metal–organic framework (MOF) [Cu3(HITP)2] (HITP = 2,3,6,7,10,11‐hexaiminotriphenylene) on hexagonal boron nitride (h‐BN) nanosheets (hereafter denoted as Cu3(HITP)2@h‐BN) for the electrocatalytic nitrogen reduction reaction (eNRR). The optimized Cu3(HITP)2@h‐BN shows the outstanding...
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