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Heme‐copper oxidase (HCO) is a class of respiratory enzymes that use a heme‐copper center to catalyze O2 reduction to H2O. While heme reduction potential (E°′) of different HCO types has been found to vary >500 mV, its impact on HCO activity remains poorly understood. Here, we use a set of myoglobin‐based functional HCO models to investigate the mechanism by which heme E°′ modulates oxidase activity...
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