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Elemental sulfur possesses an ultra‐high theoretical specific capacity, while the practical application of sulfur in lithium–sulfur (Li–S) batteries is seriously hindered by the sluggish redox kinetics and serious shuttle effect. Enhancing the catalytic activity of the sulfur host by a rational structural design is the key to address these issues. Herein, for the first time, concave‐nanocubic (CNC)...