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Experimental charge density studies of hexachloro‐cyclo‐triphosphazene (1) and the boat conformation of octachloro‐cyclo‐tetraphosphazene (2 a) were performed to unambiguously describe the origin of the electron delocalization in the P3N3 ring in 1. The obtained results were compared to DFT studies in the solid state and the gas phase. Electron density analysis revealed a highly polarized nature of...
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