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A 2,2′‐bipyridyl‐bridged tetrathiafulvalene (TTF)‐quinone dyad (1) was synthesized and characterized. Both absorption and ESR spectroscopic studies clearly indicate that electron transfer occurs from TTF to the quinone unit for dyad 1 in the presence of metal ions. The results manifest that the coordination of dyad 1 with metal ions plays a key role in facilitating the intramolecular electron transfer.
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