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More than 25 years ago, low temperature experiments aimed at establishing the ultimate limits to optical storage in solids led to the first optical detection and spectroscopy of a single molecule in the condensed phase. At this unexplored ultimate limit, many surprises occurred where single molecules showed both spontaneous changes (blinking) and light-driven control of emission, properties that were...
Single fluorescent molecules provide useful nanometer-sized absorbers and sources of light, which enable superresolution imaging, trapping, and nanometer-scale probing of optical fields in nanophotonic structures. Fundamentals of these effects will be described.
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