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A new phase-matching borate K3Sr3Li2Al4B6O20F features double-layer structure similar to that of the outstanding ultraviolet nonlinear optical material Sr2Be2B2O7, and thus inherits its excellent linear and nonlinear optical properties in some degree. Furthermore, it overcomes the structurally dynamical instability problem existing in Sr2Be2B2O7. The first-principles calculations and anionic group...
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