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A 7‐pyrrolidino‐7‐benzylamino‐8,8‐dicyanoquinodimethane, PBEDQ, (1), donor–acceptor–modified electrode yields, in the presence of hydroquinone, (2), an anodic photocurrent with quantum efficiency of 1.5%. The PBEDQ‐functionalized electrode yields, in the presence of the electron acceptor diquat, (3), a cathodic photocurrent with a quantum efficiency corresponding to 2.1%. The electron transfer cascades...
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