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Understanding the behavior of the matter under pressure is crucial for the development of novel polymorph of the chalcopyrite compound. Herein, we study the evolution of the bonding of ZnSiP2 up to 100 GPa. We particularize our results by means of the detailed ab initio study of its structural and dynamical properties. In fact, the compound shows disordered structure at 32 GPa which transforms at...
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