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Novel nonplanar bis(1,3-dithiole) donors with small on-site Coulomb repulsion afforded unusual cation radical salts as single crystals whose properties were strikingly affected by the incorporated solvent molecules.
The metal-insulator transitions occur at 190K and 20K for (BEDT-TTF) 2 MM'(SCN) 4 [M=Rb, M'=Co,Zn] and [M=Cs,M'=Co,Zn], respectively. The former transition at 190K might originate from electron-correlation with lattice modulation, suggested by the measurements of magnetic susceptibility and X-ray structure at low temperature. This transition temperature is elevated with applying pressure...
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