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Nanostructures of ternary topological insulator (TI) Bi2Te2Se are, in principle, advantageous to the manifestation of topologically nontrivial surface states, due to significantly enhanced surface‐to‐volume ratio compared with its bulk crystals counterparts. Herein, the synthesis of 2D Bi2Te2Se crystals on mica via the van der Waals epitaxy method is explored and systematically the growth behaviors...
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