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The coordination microenvironment modulation of single‐atom catalysts (SACs) based on p‐block metals holds promise for excavating their enormous potential in electrochemical CO2‐to CO conversion. Guided by the instructive theoretical calculations over serial asymmetric coordination microenvironments, herein, a novel Pb SAC with highly asymmetric coordination microenvironment (Pb‐N2SV) is developed...
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