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In this study, the authors employ synchrotron techniques to characterize multi‐scale microstructure in elucidating how the modified crystal lattices at angstrom level and molecular stacking at micrometer scale of titanium oxide phthalocyanine (TiOPc) thin film tuning the impedance. The a and c lattice lengths of the TiOPc reveal a positive correlation with the impedance because of the π‐π stacking...
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