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A fruitful stereochemical scenario of metal‐organic cages (MOCs) is demonstrated by Cheng‐Yong Su et al. in their Research Article (e202315053). Based on the intrinsic dynamics of different metal ions, it is shown how the dynamic stereochemistry of the cages is correlated with the coordination lability of the metal centers, and how their chiral induction, resolution and recognition behaviors can be...
A series of isostructural supramolecular cages with a rhombic dodecahedron shape have been assembled with distinct metal‐coordination lability (M8Pd6‐MOC‐16, M=Ru2+, Fe2+, Ni2+, Zn2+). The chirality transfer between metal centers generally imposes homochirality on individual cages to enable solvent‐dependent spontaneous resolution of Δ8/Λ8−M8Pd6 enantiomers; however, their distinguishable stereochemical...
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