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Low energy HO–CO + ions [ΔH f (298) = 142 ± 2 kcal/mol] uniquely dissociate to H–CO + + O. From ab initio molecular orbital calculations a mechanism is proposed which involves a 1,2-hydrogen shift of HO–CO + ( 1 A′) to H–CO 2+ ( 1 A′) followed by an interstate crossing leading to a transient triplet 3 A″ state which then dissociates...
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