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Time‐resolved coherent anti‐Stokes Raman spectroscopy can disentangle the exciton energy dissipation (EED) dynamics of the intrachain exciton in conjugated polymers (MEH‐PPV) coupled with several phonon modes and the corresponding phonon relaxation dynamics by adjusting the timing between lasers in the coherent anti‐Stokes Raman spectroscopy system. The intrachain EED process is coupled with phonon...
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