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Designing efficient and cost‐effective electrocatalysts is the primary imperative for addressing the pivotal concerns confronting lithium–oxygen batteries (LOBs). The microstructure of the catalyst is one of the key factors that influence the catalytic performance. This study proceeds to the advantage of metal‐organic frameworks (MOFs) derivatives by annealing manganese 1,2,3‐triazolate (MET‐2) at...