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Highly regioregular (RR) poly(3‐hexylthiophene)s PHTs are known to exhibit excellent electrical properties in comparison to chemically identical but regiorandom (rr) PHTs. In this study, distinct RR (97% and 55%)‐graded PHTs are subjected to solution blending to spontaneously separate the high‐RR PHT chains from the low‐RR PHT media and develop highly conjugated nanodomains in both solution and film...
In article number 1903163, Hoichang Yang and co‐workers demonstrate the spontaneous phase‐separation behavior of semiconducting polymer blends, such as poly(3‐hexylthiophene)s (PHTs) with different regioregularity. The simple solution blending of PHTs yields highly conjugated nanodomains including regioregular, rigid PHT chains surrounded by regiorandom, soft PHT phase in both solution and cast film,...
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