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Triplet‐excited‐state‐involved photonic and electronic properties have attracted tremendous attention for next‐generation technologies. To populate triplet states, facile intersystem crossing (ISC) for efficient exciton spin‐flipping is crucial, but it remains challenging in organic molecules free of heavy atoms. Here, a new strategy is proposed to enhance the ISC of purely organic optoelectronic...
A heteroatom‐mediated resonance activation strategy is developed by Runfeng Chen, Wei Huang, and co‐workers in article number 1803856 to dynamically enhance the spin‐flipping of purely organic molecules through the fluctuation of excited‐state energies and n‐orbital components upon resonance variation. Impressively, efficient organic ultralong room‐temperature phosphorescence with simultaneously elongated...
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