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A general and efficient rhodium‐catalyzed asymmetric cyanide‐free hydrocyanation of alkenes has been developed. Based on the asymmetric hydroformylation/condensation/aza‐Cope elimination sequences, a broad scope of substrates including mono‐substituted, 1,2‐, and 1,1‐disubstituted alkenes (involving natural product R‐ and S‐limonene) were employed, and a series of valuable chiral nitriles are prepared...
Eine asymmetrische cyanidfreie Hydrocyanierung von Alkenen wird von H. Lv, X. Zhang et al. in ihrer Zuschrift auf S. 11044 beschrieben. Auf Basis einer Sequenz aus asymmetrischer Hydroformylierung, Kondensation und Aza‐Cope‐Eliminierung wurden vielfältige Substrate, z. B. monosubstituierte sowie 1,2‐ und 1,1‐disubstituierte Alkene, eingesetzt, um eine Reihe nützlicher chiraler Nitrile in hohen Ausbeuten...
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