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A novel GrO@MIL-101 composite consisting of graphene oxide (GrO) and MIL-101(Cr) was synthesized, characterized and tested for separation of CO2/CH4 mixture. GrO@MIL-101 had higher BET surface area and better porosity than parent MIL-101. CO2 and CH4 isotherms were separately measured at different temperatures using a gravimetric method, and were fitted using the dual-site Langmuir–Freundlich (DSLF)...
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