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Novel Li/Al‐LDHs with high layer charges (HCLDHs) were synthesized in the light of the inter‐layer effect on Li+ adsorption. Compared with conventional low‐charge Li/Al‐LDHs (LCLDHs), HCLDHs exhibited a distinct micromorphology characterized by a preferential growth orientation along the c‐axis and a significantly reduced lateral diameter. Adsorption experiments showed that HCLDHs possessed superior...
Aluminum‐based lithium adsorbent (Li/Al‐LDH) is the only industrialized adsorbent for Li+ extraction from salt lake brines. The inherent mechanism of declined Li+ adsorption performance was revealed to explain the feebleness in sulfate‐type brines. SO42− in brines could replace interlayer Cl− by a stronger electrostatic attraction with laminates, significantly altering the stacking structure and interlayer...
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