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In the framework of the CALPHAD approach, a thermodynamic assessment of the metastable phases in Al–Mg–Si alloys is presented. The early Mg–Si co-clusters are described as a regular solid solution phase. A split model of fcc-based ordering is used for Guinier–Preston (GP)-zones as suggested by the assessment of microstructural data. The model parameters are optimized based on new thermodynamic first-principles...
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