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Transparent glass ceramics (GCs) consisting of an homogeneous glass phase and a well‐dispersed crystal phase are considered as ideal optical gain materials potentially applied in optoelectronic devices due to the combination of facile processability of glass and the intense crystal field of nanocrystals. Here, a heat‐induced nanocrystal‐in‐glass method is employed to integrate the active ions Tm3+...
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