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The highly trans stereoselective formation of cyclopropane derivative trans‐CP 6 via the reaction of ammonium salt (AS 2) with methyl vinyl ketone (MVK) in the presence of Na2CO3 was theoretically investigated within Molecular Electron Density Theory (MEDT) at the B3LYP/6‐31G(d) computational level to probe energetics, selectivities, and molecular mechanism. This domino reaction starts by nucleophilic...
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