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Herein, the effects of Fe/Ni ratio on the microstructure, mechanical properties, and corrosion resistance in a 3.5 wt% NaCl solution of FexNi65−xCr20Al10Nb5 are investigated systematically. It is found that the phases shifted from the FCC‐dominated to the BCC‐dominated with the molar ratio of the Fe/Ni increased. The strength of FexNi65−xCr20Al10Nb5 increases with the molar ratio of Fe/Ni further...