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We report a photodetachment and high-resolution photoelectron imaging study of cold deprotonated 2-hydroxypyrimidine anions, C4H3N2O−. Photodetachment spectroscopy reveals an excited dipole-bound state (DBS) of C4H3N2O− with a binding energy of 598±5cm−1 below the detachment threshold of 26,010±5cm−1. Twenty vibrational levels of the DBS are observed as resonances in the photodetachment spectrum,...
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