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Quinones exhibit orthogonal ground‐ and excited‐state reactivities and are therefore highly suitable organocatalysts for the development of sequential catalytic processes. Herein, the discovery of an anthraquinone‐catalyzed thermal indole‐C3‐alkylation with benzylamines is described, which can be combined sequentially with a new visible‐light‐driven catalytic photooxidation/1,2‐shift reaction. The...
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