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Complexes [M(P,SR)(diene)X] where (P,SR)=CpFe[1,2-C5H3(PPh2)(CH2SR)] (M=Ir, R=tBu or Bn diene=cod, X=Cl; M=Rh, diene=cod or nbd; X=BF4 or Cl) were used as precatalysts for the redox isomerization of various allylic alcohols (7a–e) to the corresponding saturated ketones (8a–e) and or hydrogenation to the saturated alcohol (9a–e). In optimization studies using 1-phenyl-2-propen-1-ol (7a) in THF and...
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