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The polypyrazolyl ligand H4L, a functionalised derivative of 3‐bpp [bpp = bis(pyrazol‐3‐yl)pyridine], has been used to synthesise an FeII spin‐crossover (SCO) system [Fe(H4L)2](ClO4)2·2THF·H2O (1). A subsequent magnetic and structural study revealed that the compound undergoes an incomplete transition with a small hysteresis loop of 8 K and a large residual high spin (HS) fraction. This is consistent...
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