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Selective excitation of parent modes and detection of the intramolecular vibrational energy flow to daughter modes is proposed by the femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) spectroscopy. Vibrational modes of CCN bending at 379 cm−1, CN stretching at 2253 cm−1 and CH stretching at 2943 cm−1 are excited, energy flow to relative higher frequency ones located outside the...
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