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Hybrid organic–inorganic perovskite (HOIP) ferroelectric materials have great potential for developing self‐powered electronic transducers owing to their impressive piezoelectric performance, structural tunability and low processing temperatures. Nevertheless, their inherent brittle and low elastic moduli limit their application in electromechanical conversion. Integration of HOIP ferroelectrics and...
Helicobacter pylori (H. pylori) is the major etiological factor of a variety of gastric diseases. However, the treatment of H. pylori is challenged by the destruction of targeted drugs by gastric acid and pepsin. Herein, a dual‐targeted cascade catalytic nanozyme PtCo@Graphene@Hemin‐2(L‐arginine) (PtCo@G@H2A) is designed for the treatment of H. pylori. The dual‐targeting ability of PtCo@G@H2A is derived...
Organic–inorganic hybrid lead halide perovskites (OLHPs), represented by (CH3NH3)PbI3, are one of the research focus due to their exceptional performance in optoelectronic applications, and ferroelastic domain walls are benign to their charge carrier transport that is confirmed recently. Among them, the 1D OLHPs feature better stability against desorption and moisture, but related 1D ones possessing...
Utilization of life‐like hydrogels to replicate synergistic shape/color changeable behaviors of living organisms has been long envisaged to produce robust functional integrated soft actuators/robots. However, it remains challenging to construct such hydrogel systems with integrated functionality of remote, localized and environment‐interactive control over synergistic discoloration/actuation. Herein,...
Increasing the fill factor (FF) and the open‐circuit voltage (VOC) simultaneously together with non‐decreased short‐circuit current density (JSC) are a challenge for highly efficient Cu2ZnSn(S,Se)4 (CZTSSe) solar cells. Aimed at such target in CZTSSe solar cells, a synergistic strategy to tailor the recombination in the bulk and at the heterojunction interface has been developed, consisting of atomic‐layer...
Bi Doped Graphene
In article number 2206218, Xianyang Lu, Thomas Frauenheim, Yongbing Xu, and co‐workers investigate femtosecond laser excitation induced electronic dynamic in Bi doped graphene, using time resolved and angular resolved photoemission spectrum. The Fermi surface in Dirac cone and carrier concentration is modulated by adatoms' content. This effectively tailors the competition between...
By introducing different contents of Bi adatoms to the surface of monolayer graphene, the carrier concentration and their dynamics have been effectively modulated as probed directly by the time‐ and angle‐resolved photoemission spectroscopy technique. The Bi adatoms are found to assist acoustic phonon scattering events mediated by supercollisions as the disorder effectively relaxes the momentum conservation...
About 10% efficient antimony selenosulfide (Sb2(S,Se)3) solar cell is realized by using selenourea as a hydrothermal raw material to prepare absorber layers. However, tailoring the bandgap of hydrothermal‐based Sb2(S,Se)3 film to the ideal bandgap (1.3–1.4 eV) using the selenourea for optimal efficiency is still a challenge. Moreover, the expensive selenourea dramatically increases the fabricating...
Supported bimetallic nanoparticles (NPs) with ultrasmall sizes and homogeneous alloying are attractive for catalysis. However, facile synthesis of this type of material remains very challenging. Here, the aerosol drying impregnation method for rapid, scalable, and general synthesis of silica‐supported bimetallic NPs is proposed. The method relies on aerosol spray drying to promote the mixing and dispersing...
Aqueous zinc (Zn) metal batteries have been regarded as the most promising aqueous batteries due to their low redox potential, high theoretical capacity, and abundant Zn resources. Unfortunately, Zn dendrite growth and serious side reactions drastically curtail the cycle life, severely affecting their large‐scale application. Herein, a multifunctional ordered Zn‐aminotrimethylene phosphonic acid (Zn‐ATMP)...
Nanofluidics
In article number 2102150, Hui Yang and co‐workers report a high‐throughput nanofluidic device for loading of various cargos into exosomes. The exosomes treated by the device can deliver their drug cargos to cancer cells and induce cell death, indicating the potential opportunities of the device for developing new exosome‐based delivery vehicles for further biomedical applications.
Efficient loading of various exogenous cargos into exosomes while not affecting their integrity and functionalities remains a major challenge. Here, a nanofluidic device named “exosome nanoporator (ENP)” is presented for high‐throughput loading of various cargos into exosomes. By transporting exosomes through nanochannels with height comparable to their dimension, exosome membranes are permeabilized...
Interfacial engineering methods have been developed to solve defect issues of perovskite solar cells (PSCs). However, traditional surface passivation has limited effects on eliminating defect‐forming residuals, while secondary grain growth (SGG) is restricted by limited choices of additives and intrinsic properties of perovskites. Here, a pincer strategy of taking advantages of surface passivation...
Materials exhibiting persistent luminescence (PersL) have great prospect in optoelectronic and biomedical applications such as optical information storage, bio‐imaging, and so on. Unfortunately, PersL materials with multimode emission properties have been rarely reported, although they are expected to be very desirable in multilevel anti‐counterfeiting and encryption applications. Herein, Cr3+‐doped...
Bolometric photodetectors have been widely investigated and studied since their delicate applications in military, commercial, public, and academic domains. In article number 1904482, Hailin Peng, Xueao Zhang, Shiqiao Qin, and co‐workers report that a Bi2O2Se‐based bolometer shows a high temperature coefficient of resistance (−1.6% K−1), high bolometric coefficient (−31 nA K−1) and high bolometric...
Bi2O2Se is emerging as a photosensitive functional material for optoelectronics, and its photodetection mechanism is mostly considered to be a photoconductive regime in previous reports. Here, the bolometric effect is discovered in Bi2O2Se photodetectors. The coexistence of photoconductive effect and bolometric effect is generally observed in multiwavelength photoresponse measurements and then confirmed...
The atomic structure of free‐standing graphene comprises flat hexagonal rings with a 2.5 Å period, which is conventionally considered the only atomic period and determines the unique properties of graphene. Here, an unexpected highly ordered orthorhombic structure of graphene is directly observed with a lattice constant of ≈5 Å, spontaneously formed on various substrates. First‐principles computations...
In article number 1902637, Guosheng Shi, Yi Zhang, and co‐workers discover an orthorhombic crystal of graphene with an ≈5 Å period formed on various substrates, which can be applied to control the epitaxial self‐assembly of amyloid peptides. First‐principle computations show that this atomic structure can be attributed to dipoles between the graphene surface and substrates.
2D β‐Ga2O3 nanosheets, as fundamental materials, have great potential in next generations of ultraviolet transparent electrodes, high‐temperature gas sensors, solar‐blind photodetectors, and power devices, while their synthesis and growth with high crystalline quality and well‐controlled orientation have not been reported yet. The present study demonstrates how to grow single‐crystalline ultrathin...
Using interfacial reaction systems for biphasic catalytic reactions is attracting more and more attention due to their simple reaction process and low environmental pollution. Yolk–shell structured materials have broad applications in biomedicine, catalysis, and environmental remediation owing to their open channels and large space for guest molecules. Conventional methods to obtain yolk–shell mesoporous...
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