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Treatment of meso‐chlorosubporphyrin with controlled equivalents of Na2S·9H2O in DMF led to the formation of either meso‐to‐meso sulfide (S)‐bridged dimer 4 or disulfide (SS)‐bridged subporphyrin dimer 6. S‐bridged dimer 4 displayed a split Soret‐like band and a large Stokes shift and became a fully delocalized one‐quantum system in the S1 state, as indicated by femtosecond transient absorption anisotropy...
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