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Systematic reaction path exploration revealed the entire mechanism of Knowles's light‐promoted catalytic intramolecular hydroamination. Bond formation/cleavage competes with single electron transfer (SET) between the catalyst and substrate. These processes are described by adiabatic processes through transition states in an electronic state and non‐radiative transitions through the seam of crossings...
Systematic reaction path exploration revealed the entire mechanism of Knowles’ light‐promoted catalytic intramolecular hydroamination via radical processes. In their Research Article (e202211936), Yu Harabuchi, Satoshi Maeda, and co‐workers investigated the energetically favorable reaction path by constructing reaction path networks and searching for the seam of crossing geometries. Calculations showed...
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