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Phosph(III)azanes, featuring the heterocyclobutane P2N2 ring, have now been established as building blocks in main‐group coordination and supramolecular compounds. Previous studies have largely involved their use as neutral P‐donor ligands or as anionic N‐donor ligands, derived from deprotonation of amido‐phosphazanes [RNHP(μ‐NR)]2. The use of neutral amido‐phosphazanes themselves as chelating, H‐bond...
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