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Herein, we report a practical two‐step synthetic route to α‐arylpyrrolidines through Suzuki–Miyaura cross‐coupling and enantioselective copper‐catalyzed intramolecular hydroamination reactions. The excellent stereoselectivity and broad scope for the transformation of substrates with pharmaceutically relevant heteroarenes render this method a practical and versatile approach for pyrrolidine synthesis...
Die erste mehrstufige asymmetrische Katalyse in einem Strömungsreaktor wurde durch einer Sequenz aus Lithiierung, Borylierung und Rhodium‐katalysierter 1,4‐Addition realisiert. Die dreistufige Sequenz geht von einfach erhältlichen, preiswerten Arylbromiden aus und liefert β‐arylierte Ketone in guten Ausbeuten und mit hohen Enantioselektivitäten.
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