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Strontium and calcium (alkaline earth: Ae) olefin complexes stabilised by secondary Ae⋅⋅⋅F−C and β‐agostic Ae⋅⋅⋅H−Si interactions are presented. Olefin coordination onto the alkaline earths is plain in the solid state, and it is thermodynamically favoured over the coordination of THF. The existence of the Ae⋅⋅⋅olefin interactions is corroborated by solution NMR data and DFT computations. The coordination...
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