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Chiral monodentate phosphines based on ortho‐disubstituted ferrocene units have been prepared and used for the synthesis of gold(I) complexes. These complexes are highly active catalysts for the cycloisomerization of 3‐hydroxy‐1,5‐enynes into bicyclo[3.1.0]hexanones. Their high catalytic activity is ascribed to their structural analogy to the biaryl‐based Buchwald phosphines. This paper discloses...
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