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The single copper atom doped clusters CuAl4O7–9− can catalyze CO oxidation by O2. The CuAl4O7–9− clusters are the first group of experimentally identified noble‐metal free single atom catalysts for such a prototypical reaction. The reactions were characterized by mass spectrometry and density functional theory calculations. The CuAl4O9CO− is much more reactive than CuAl4O9− in the reaction with CO...
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