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Catalytic desaturations are important strategies for the functionalization of organic molecules. In nature, flavoenzymes mediate the formation of α,β‐unsaturated carbonyl compounds by concomitant cofactor reduction. Contrary to many laboratory methods for these reactions, such as the Saegusa‐Ito oxidation, no transition metal reagents or catalysts are required. However, a molecular flavin‐mediated...
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