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Regulating the second sphere of homogeneous molecular catalysts is a common and effective method to boost their catalytic activities, while the second sphere effects have rarely been investigated for heterogeneous single‐atom catalysts primarily due to the synthetic challenge for installing functional groups in their second spheres. Benefiting from the well‐defined and readily tailorable structure...
Regulating the second sphere of homogeneous molecular catalysts is a common and effective method to boost their catalytic activities, while the second sphere effects have rarely been investigated for heterogeneous single‐atom catalysts primarily due to the synthetic challenge for installing functional groups in their second spheres. Benefiting from the well‐defined and readily tailorable structure...
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