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Rechargeable lithium‐metal batteries (RLBs), which employ the Li‐metal anode to acquire notably boosted specific energy at cell level, represent the “Holy Grail” for “beyond Li‐ion” electrochemical energy storage technology. Currently, the practical use of RLBs is impeded by poor cycling and safety performance, which are derived from high chemical reactivity of metallic Li and uncontrollable formation...