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In this work, a novel version of macrocyclic arenes, namely leaning pillar[6]arenes, was discovered and it can be considered as a tilted version of a pillar[6]arene with two hydroxy/alkoxy functionalities removed. Through a facile two‐step synthetic approaches, in conjunction with a diversity of post‐modification possibilities, a series of leaning pillar[6]arenes, with good cavity adaptability and...
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